Journal
NANOMATERIALS
Volume 11, Issue 4, Pages -Publisher
MDPI
DOI: 10.3390/nano11040959
Keywords
quantum dots (QDs); ZnO nanoparticles; solvent optimization; quantum dot light-emitting diodes (QLEDs)
Categories
Funding
- Natural Science Foundation of Jiangsu Province [BK20190774]
- National Key R&D Program of China [2017YFC0111500, 2016YFB0401600]
- National Natural Science Foundation Project [61775034, 61571124, 61674029, 61875082, U1804132]
- Jiangsu Province College Graduate Research Innovation Program [KYCX19_0082]
- Research Start-Up Fund of NUIST [2019r035]
- Priority Academic Program Development of Jiangsu Higher Education Institutions
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In this study, high-performance blue quantum dots light-emitting diodes using ZnO nanoparticles as the electron transport layer were reported. Experimental results showed that the properties of solvents used for ZnO NPs play a crucial role in modulating electron injection across the QDs/ETL interface. Blue QLEDs with ZnO NPs dispersed in butanol exhibited significantly improved current efficiency and external quantum efficiency compared to other solvents.
Here, we report on the high-performance blue quantum dots (QDs) light-emitting diodes (QLEDs), in which the ZnO nanoparticles (NPs) are employed as the electron transport layer (ETL) and optimized with different alcohol solvents. The experimental results demonstrate that the properties of solvent used for ZnO NPs-such as polarity, viscosity and boiling point-play a crucial role in the quality of film where they modulate the electron injection across the QDs/ETL interface. The maximum current efficiency of 3.02 cd/A and external quantum efficiency (EQE) of 3.3% are achieved for blue QLEDs with ZnO NPs dispersed in butanol, exhibiting obvious enhancement compared with the other solvents. This work provides a new method to select proper solvent for ETL which can further improve the device performance.
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