4.7 Article

Multifunctional molybdenum disulfide flash memory using a PEDOT:PSS floating gate

Journal

NPG ASIA MATERIALS
Volume 13, Issue 1, Pages -

Publisher

NATURE RESEARCH
DOI: 10.1038/s41427-021-00307-x

Keywords

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Funding

  1. National Research Foundation of Korea [2018R1A2B2003558]
  2. Basic Science Research Program through the National Research Foundation of Korea - Ministry of Education [2020R1I1A1A01070907, 2020R1I1A1A01073884]
  3. National Research Foundation of Korea (NRF) - Korean government (MSIT) [2020M3A9E4104385, 2020R1A2C1101647]
  4. National Research Foundation of Korea [2020R1A2C1101647, 2020R1I1A1A01070907, 2018R1A2B2003558, 2020M3A9E4104385, 2020R1I1A1A01073884] Funding Source: Korea Institute of Science & Technology Information (KISTI), National Science & Technology Information Service (NTIS)

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The study presents a novel concept for multifunctional MoS2 flash memory, combining MoS2 with PEDOT:PSS floating layer, demonstrating high switching ratio, large memory window, and endurance. The integration of PEDOT:PSS allows for embedding the memory on a polyimide substrate, providing high mechanical endurance.
Two-dimensional transition metal dichalcogenide materials (TMDs), such as molybdenum disulfide (MoS2), have been considered promising candidates for future electronic applications owing to their electrical, mechanical, and optical properties. Here, we present a new concept for multifunctional MoS2 flash memory by combining a MoS2 channel with a PEDOT:PSS floating layer. The proposed MoS2 memory devices exhibit a switching ratio as high as 2.3 x 10(7), a large memory window (54.6 +/- 7.80 V), and high endurance (>1,000 cycles). As the PEDOT:PSS film enables a low-temperature solution-coating process and mechanical flexibility, the proposed P-memory can be embedded on a polyimide substrate over a rigid silicon substrate, offering high mechanical endurance (over 1,000 cycle bending test). Furthermore, both MoS2 and PEDOT:PSS have a bandgap that is desirable in optoelectronic memory operation, where charge carriers are stored differently in the floating gate depending on light illumination. As a new application that combines photodiodes and memory functions, we demonstrate multilevel memory programming based on light intensity and color.

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