Journal
ADVANCED ENERGY MATERIALS
Volume 11, Issue 20, Pages -Publisher
WILEY-V C H VERLAG GMBH
DOI: 10.1002/aenm.202100154
Keywords
metal‐ ion batteries; metal– organic frameworks; porosity; porous materials; supercapacitors
Categories
Funding
- EU Horizon 2020 SABYDOMA Programme [862296]
- RGG-EU Collaborative Programme initiative [E-HKU704/19]
- National Natural Science Foundation of China [51602226]
- Natural Science Foundation of Zhejiang Province [LY19E020008]
- Qingshan Lake SciTech City
- Hong Kong Quantum AI Lab Ltd - AIR@InnoHK
- URC Platform Technology Fund
- University of Hong Kong
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Metal-organic frameworks (MOFs) provide great potential for electrochemical energy storage (EES) applications due to their rich chemistry and uniformly distributed active sites. Through design and engineering, their scope of applications can be expanded, with potential uses in supercapacitors and metal-ion batteries.
Metal-organic frameworks (MOFs) feature rich chemistry, ordered micro-/mesoporous structure and uniformly distributed active sites, offering great scope for electrochemical energy storage (EES) applications. Given the particular importance of porosity for charge transport and catalysis, a critical assessment of its design, formation, and engineering is needed for the development and optimization of EES devices. Such efforts can be realized via the design of reticular chemistry, multiscale pore engineering, synthesis methodologies, and postsynthesis treatment, which remarkably expand the scope of applications. By imparting conductive backbones, guest compounds, and/or redox-active centers, MOFs and their derivatives have been heavily explored for EES in the last decade. To improve the design of MOF-based materials for EES, the strategies of pore architecturing of MOFs and their derivatives are systematically analyzed and their applications reviewed for supercapacitors and metal-ion batteries. Potential challenges and future opportunities are also discussed to guide future development.
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