4.8 Article

Near-Perfect Absorption of Light by Coherent Plasmon-Exciton States

Journal

NANO LETTERS
Volume 21, Issue 9, Pages 3864-3870

Publisher

AMER CHEMICAL SOC
DOI: 10.1021/acs.nanolett.1c00389

Keywords

Plasmonics; hot-charge carriers; ultrafast spectroscopy; strong coupling

Funding

  1. JSPS KAKENHI [JP18H05205, JP18K05053, JP20K15113]
  2. Nanotechnology Platform (Hokkaido University)
  3. Dynamic Alliance for Open Innovation Bridging Human, Environment and Materials (Five-Star Alliance) of MEXT
  4. ARC [FT140100514, DP160100983]

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We experimentally demonstrate and theoretically study the formation of coherent plasmon-exciton states, which exhibit high absorption of incident light and cancellation of absorption. Our research shows the potential implications of these coherent states and opens the prospect for devices exploiting coherent effects in applications.
We experimentally demonstrate and theoretically study the formation of coherent plasmon-exciton states which exhibit absorption of >90% of the incident light (at resonance) and cancellation of absorption. These coherent states result from the interaction between a material supporting an electronic excitation and a plasmonic structure capable of (near) perfect absorption of light. We illustrate the potential implications of these coherent states by measuring the charge separation attainable after photoexcitation. Our study opens the prospect for realizing devices that exploit coherent effects in applications.

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