4.8 Article

Nanoimaging of Low-Loss Plasmonic Waveguide Modes in a Graphene Nanoribbon

Journal

NANO LETTERS
Volume 21, Issue 7, Pages 3106-3111

Publisher

AMER CHEMICAL SOC
DOI: 10.1021/acs.nanolett.1c00276

Keywords

Graphene nanoribbon; Plasmonic waveguide modes; Near-field nanoscopy; Photonic circuit

Funding

  1. U.S. Department of Energy, Office of Science, Basic Energy Sciences, Materials Sciences and Engineering Division [DE-AC02-05-CH11231, KC2207]
  2. Office of Naval research (MURI Award) [N00014-16-1-2921]
  3. Elemental Strategy Initiative by the MEXT, Japan [JPMXP0112101001]
  4. JSPS KAKENHI [JP20H00354]
  5. CREST, JST [JPMJCR15F3]

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Graphene nanoribbons with low edge roughness fabricated using dry lithography method support low-loss and tunable plasmonic waveguide modes, which were observed using cryogenic infrared nanoscopy and can be adjusted through electrostatic gating.
Graphene nanoribbons are predicted to support low-loss and tunable plasmonic waveguide modes with an ultrasmall mode area. Experimental observation of the plasmonic waveguide modes in graphene nanoribbons, however, is challenging because conventional wet lithography has difficulty creating a clean graphene nanoribbon with a low edge roughness. Here, we use a dry lithography method to fabricate ultraclean and low-roughness graphene nanoribbons, which are then encapsulated in hexagonal boron nitride (hBN). We demonstrate low-loss plasmon propagation with a quality factor up to 35 in the ultraclean nanoribbon waveguide using cryogenic infrared nanoscopy. In addition, we observe both the fundamental and the higher-order plasmonic waveguide modes for the first time. All the plasmon waveguide modes can be tuned through electrostatic gating. The observed tunable plasmon waveguide modes in ultraclean graphene nanoribbons agree well with the finite-difference time-domain (FDTD) simulation results. They are promising for reconfigurable photonic circuits and devices at a subwavelength scale.

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