Journal
MATERIALS TODAY
Volume 50, Issue -, Pages 418-441Publisher
ELSEVIER SCI LTD
DOI: 10.1016/j.mattod.2021.03.013
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Funding
- National Natural Science Foundation of China [11765010]
- National Key Research and Development Program of China [2019YFC1907900]
- Applied Basic Research Programs of Yun-nan Provincial Science and Technology Department [202001AW070004]
- Freely Exploring Fund for Academicians in Yunnan Province [2018HA006]
- Key Laboratory of Resource Chemistry, Ministry of Education [KLRC_ME2001]
- U.S. Department of Energy (DOE) , Office of Energy Efficiency and Renewable Energy, Vehicle Technologies Office under US-China Clean Energy Research Centre (CERC-CVC2) program
- DOE Office of Science [DE-AC02-06CH11357]
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Solid-state Li-ion batteries (SSLBs) are promising next-generation energy storage devices with high energy density and enhanced safety. The solid-state electrolyte (SSE) is a key component for delivering the desired electrochemical performance characteristics. LGPS-type and garnet-type Li ion conductors are representative solid-state electrolytes that provide insights for future design and discovery of favorable solid-state Li-ion electrolytes for SSLBs. Recent advances in strategies to address the SSLB challenges have been discussed, along with a perspective on the future research directions of SSLBs.
Solid-state Li-ion batteries (SSLBs) are promising next-generation energy storage devices with high energy density and enhanced safety. The solid-state electrolyte (SSE) is a key component for delivering the desired electrochemical performance characteristics. This article provides a brief review of the discovery, synthesis, structure, ion-conduction mechanism, and application of LGPS-type and garnet-type Li ion conductors as two representative SSEs, aiming to extract principles for the future design and discovery of favourable solid-state Li-ion electrolytes for SSLBs. Recent advances in strategies to address the SSLB challenges are also discussed. Finally, a perspective on the future research directions of SSLBs is provided.
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