Journal
EUROPEAN JOURNAL OF INORGANIC CHEMISTRY
Volume -, Issue 27, Pages 4358-4362Publisher
WILEY-V C H VERLAG GMBH
DOI: 10.1002/ejic.201600064
Keywords
Metal-organic frameworks; Heterogeneous catalysis; Homogeneous catalysis; Photochemistry; Carbon dioxide reduction
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Funding
- National Natural Science Foundation of the P.R. China [21471126]
- National Thousand Talents Program of the P.R. China
- 985 Program of Chemistry and Chemical Engineering Disciplines of Xiamen University
- US National Science Foundation (NSF) [DMR-1308229]
- China Scholarship Council
- Division Of Materials Research
- Direct For Mathematical & Physical Scien [1308229] Funding Source: National Science Foundation
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A metal-organic framework (MOF) based on (bpy)Re(CO)(3)Cl-containing elongated dicarboxylate ligands and Zr-6(mu(3)-O)(4)(mu(3)-OH)(4) clusters was synthesized and used as an effective single-site catalyst to photochemically reduce carbon dioxide to carbon monoxide and formate and to provide mechanistic insights into the photocatalytic CO2 reduction process.
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