4.6 Article

Interface engineering for high-efficiency perovskite solar cells

Journal

JOURNAL OF APPLIED PHYSICS
Volume 129, Issue 13, Pages -

Publisher

AIP Publishing
DOI: 10.1063/5.0038073

Keywords

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Funding

  1. National Key Research and Development Program of China [2019YFE0101300]
  2. Natural Science Foundation of China (NSFC) [21975088]
  3. NSFC Major International (Regional) Joint Research Project NSFCSNSF [51961165106]
  4. Central Universities of Huazhong University of Science Technology [2018KFYXKJC034, 2019kfyRCPY040]
  5. Double first-class research funding of China-EU Institute for Clean and Renewable Energy [3011187029]

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This article discusses some suggestions to improve carrier transfer and reduce recombination loss for highly efficient perovskite solar cells, including primary requests on charge carrier transfer dynamics, reasonable design methodologies, and tuning interface interaction between perovskite and charge transport layers.
The power conversion efficiency of thin film solar cells using organic-inorganic hybrid lead halide perovskite as an absorber has achieved over 25%. An augment of the output voltage can further increase the efficiency approaching the Shockley-Queisser efficiency limitation, which is highly correlated with charge carrier management at interfaces in perovskite devices. This perspective presents some considerations to improve carrier transfer and reduce recombination loss for highly efficient perovskite solar cells, including primary requests on charge carrier transfer dynamics, reasonable design methodologies of interfacial materials, and tuning interface interaction between perovskite and charge transport layers.

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