4.7 Article

Life-Cycle Environmental and Economic Assessments of the Oxy- coal Combustion System Combined with a Pressurized Circulating Fluidized Bed and the Supercritical CO2 Brayton Cycle

Journal

ENERGY & FUELS
Volume 35, Issue 10, Pages 8868-8883

Publisher

AMER CHEMICAL SOC
DOI: 10.1021/acs.energyfuels.1c00067

Keywords

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Funding

  1. National Natural Science Foundation of China [51736002]

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By conducting a comprehensive life-cycle environmental and economic assessment of oxy-coal combustion with circulating fluidized bed power plants with a pressurized combustor and a supercritical CO2 Brayton cycle, it was found that the systems have lower damage to human health and the environment, as well as relatively lower costs of electricity, CO2 capture, and CO2 avoidance. The study also discusses the impact of various parameters on economic indicators.
Oxy-coal combustion with circulating fluidized bed (OCFB) is a promising technology for CO2 capture and sequestration. However, its development is highly hindered by the high price of electricity and CO2 capture. In this work, a comprehensive life-cycle environmental and economic assessment of OCFB power plants with a pressurized combustor (POCFB) and a supercritical CO2 Brayton cycle is conducted using a specific life-cycle assessment (LCA) method. There are four processes evaluated in this work, including construction material production, transport, raw material mining, and power plant operation. Both environmental midpoint and endpoint impacts are derived and compared. The results show that compared to the oxy-coal combustion power plant, systems with a pressurized combustor and a S-CO2 Brayton cycle have less damage (6-12%) to the human health and the environment. Meanwhile, compared to the OCFB power plant, POCFB has relatively lower costs of electricity, CO2 capture, and CO2 avoidance, which are 58.1 USD/MWh, 15.5 USD/t, and 33.4 USD/t, respectively. The results from the Analytic Hierarchy Process-Technique for Order Preference by Similarity to Ideal Solution methodology show that comprehensively considering the economy, resource, and environment, the POCFB power plant is the best option among the cases from the perspective of residents and the government. The influence of several parameters including net electricity efficiency, CO2 capture rate, boiler investment, coal price, and CO2 tax on the economic indicators is also discussed.

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