Journal
CHEMISTRY-AN ASIAN JOURNAL
Volume 16, Issue 10, Pages 1229-1232Publisher
WILEY-V C H VERLAG GMBH
DOI: 10.1002/asia.202100244
Keywords
palladium; hydrogenation; ketone; valerolactone; levulinic acid
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Funding
- National Natural Science Foundation of China [21961045, 21572198, 22061048]
- Applied Basic Research Project of Yunnan Province [2017FA004, 2018FB021]
- Yunnan Provincial Key Laboratory Construction Plan Funding of Universities
- Yunnan Provincial Engineering Research Center Construction Plan Funding of Universities
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This study has successfully developed a palladium-catalyzed asymmetric hydrogenation of levulinic acid using Zn(OTf)(2) as co-catalyst, providing a new strategy in the field of palladium-catalyzed asymmetric hydrogenation of ketones. It allows the preparation of a wide range of chiral gamma-valerolactones in good yields with excellent enantioselectivities.
A palladium-catalyzed asymmetric hydrogenation of levulinic acid has been successful developed by using Zn(OTf)(2) as co-catalyst. The present method not only has provided a strategy in the palladium-catalyzed asymmetric hydrogenation of ketone, but also allowed the preparation of a wide range of chiral gamma-valerolactones in good yields with excellent enantioselectivities.
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