4.7 Article

Fabrication of Nd-doped Ni-Zn ferrite/multi-walled carbon nanotubes composites with effective microwave absorption properties

Journal

CERAMICS INTERNATIONAL
Volume 47, Issue 8, Pages 10545-10554

Publisher

ELSEVIER SCI LTD
DOI: 10.1016/j.ceramint.2020.11.137

Keywords

Ferrite; Earth elements doped; Multi-walled carbon nanotubes; Microwave absorption properties

Funding

  1. National Natural Science Foundation of China [51702158]
  2. Key Laboratory of Materials Preparation and Protection for Harsh Environment (Nanjing University of Aeronautics and Astronautics) , Ministry of Industry and Information Technology [56XCA1901305]

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The study successfully synthesized a new type of MWCNTs/Ni0.5Zn0.5Nd0.04Fe1.96O4 composites, and the addition of MWCNTs significantly improved the microwave absorption performance, enhancing the microwave attenuation performance and impedance matching coefficient of the electromagnetic materials.
The electromagnetic materials are featured by good magnetic permeability and dielectric constant characteristics, which are of significant importance in solving the pollution problem of electromagnetic. In this study, after the complete of the use of sol-gel method, argon gas was then introduced for calcination, and eventually a new type of MWCNTs/Ni0.5Zn0.5Nd0.04Fe1.96O4 composites was synthesized after the above mentioned procedures. The synthesized MWCNTs were able to be adsorbed on the surface of Ni0.5Zn0.5Nd0.04Fe1.96O4 and could form a good conductive work of 3D. Also, the effect of additional MWCNTs on microwave absorption properties of MWCNTs/Ni0.5Zn0.5Nd0.04Fe1.96O4 composites were also observed in this study. The results indicate that the additional MWCNTs function to significantly improve the microwave absorption property of MWCNTs/ Ni0.5Zn0.5Nd0.04Fe1.96O4. Through altering the amount of MWCNTs, the microwave attenuation performance and impedance matching coefficient of this electromagnetic materials can be effectively improved. The S2 sample presented a minimum reflection loss of -35.05 dB when its thickness reached 1.6 mm, meanwhile, the effective absorption bandwidth achieved 4.55 GHz. The prepared composites perform well in microwave absorption, which can attribute to the reasonable ratio of composites as well as its interaction with both of the magnetic and dielectric components. This research paved the way for novel ideas to be put in the electromagnetic absorption materials with high-efficient.

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