Journal
ADVANCED MATERIALS
Volume 33, Issue 18, Pages -Publisher
WILEY-V C H VERLAG GMBH
DOI: 10.1002/adma.202100484
Keywords
chaotic lasing; crystal growth; organic lasers; organic nanophotonics; organic semiconductors
Categories
Funding
- Ministry of Science and Technology of China [2017YFA0204502]
- National Natural Science Foundation of China [21790364, 51903238]
- Postdoctoral Innovation Talent Support Project [BX20180314]
- China Postdoctoral Science Foundation [2019M650854]
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Novel mesoscopic semiconductor architectures are continuously synthesized using a superkinetic crystal growth method to produce 2D oval organic semiconductor microcrystals. These microcrystals break the crystal growth anisotropy and naturally form chaotic optical microresonators, supporting low-threshold lasing and directional laser emission assisted by chaotic modes. These results will reshape crystal growth theory understanding and guide the design of crystalline photonic materials.
Synthesis of novel mesoscopic semiconductor architectures continually generates new photonic knowledge and applications. However, it remains a great challenge to synthesize semiconductor microcrystals with smoothly curved surfaces owing to the crystal growth anisotropy. Here, a superkinetic crystal growth method is developed to synthesize 2D oval organic semiconductor microcrystals. The solid source dispersion induces an exceptionally large molecular supersaturation for vapor deposition, which breaks the crystal growth anisotropy. The synthesized stadium-shaped organic semiconductor microcrystals naturally constitute fully chaotic optical microresonators. They support low-threshold lasing on high-quality-factor scar modes localized near the stadium boundary and directional laser emission assisted by the chaotic modes. These results will reshape the understanding of the crystal growth theory and provide valuable guidance for crystalline photonic materials design.
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