Journal
ADVANCED MATERIALS
Volume 33, Issue 50, Pages -Publisher
WILEY-V C H VERLAG GMBH
DOI: 10.1002/adma.202005484
Keywords
catalysts; CO; (2) reduction; electrocatalysis; structural; compositional effects
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Funding
- Research Grant Council of the Hong Kong Special Administrative Region [16310419, 16309418]
- Innovation and Technology Commission of the Hong Kong Special Administrative Region [ITC-CNERC14EG03]
- Research Grant Council Postdoctoral Fellowship Scheme of the Hong Kong Special Administrative Region [PDFS2021-6S08]
- Jiangsu Key Laboratory for the Chemistry of Low-Dimensional Materials [JSKC19016]
- Hong Kong Scholars Program [XJ2019042]
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This study summarized the recent advances in using advanced electrocatalysts for electrochemical CO2 reduction, as well as strategies to regulate the selectivity and activity of CO2 reduction, and discussed future research directions.
Electrochemical CO2 reduction has been recognized as a promising solution in tackling energy- and environment-related challenges of human society. In the past few years, the rapid development of advanced electrocatalysts has significantly improved the efficiency of this reaction and accelerated the practical applications of this technology. Herein, representative catalyst structures and composition engineering strategies in regulating the CO2 reduction selectivity and activity toward various products including carbon monoxide, formate, methane, methanol, ethylene, and ethanol are summarized. An overview of in situ/operando characterizations and advanced computational modeling in deepening the understanding of the reaction mechanisms and accelerating catalyst design are also provided. To conclude, future challenges and opportunities in this research field are discussed.
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