4.8 Review

Switched-On: Progress, Challenges, and Opportunities in Metal Halide Perovskite Transistors

Journal

ADVANCED FUNCTIONAL MATERIALS
Volume 31, Issue 29, Pages -

Publisher

WILEY-V C H VERLAG GMBH
DOI: 10.1002/adfm.202101029

Keywords

field‐ effect transistors; hysteresis; perovskites; phototransistors; stability

Funding

  1. European Research Council (ERC) under the European Union's Horizon 2020 research and innovation program (ERC) [714067]
  2. Deutsche Forschungsgemeinschaft (DFG) [SPP 2196, VA 991/3-1, DE 830/22-1, VA 991/2-1]
  3. National Science Foundation [1608095, 1810273]
  4. Projekt DEAL
  5. Directorate For Engineering
  6. Div Of Electrical, Commun & Cyber Sys [1608095] Funding Source: National Science Foundation
  7. Div Of Electrical, Commun & Cyber Sys
  8. Directorate For Engineering [1810273] Funding Source: National Science Foundation

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This review discusses the current status of field-effect transistors, the success of metal halide perovskite materials in photovoltaics, and the exploration of their application in other optoelectronic devices. It also highlights the challenges and provides an outlook for the future perspectives of perovskite FETs. The role of ion migration, defects, temperature, light, and measurement conditions in influencing these devices is examined, along with a survey and critical assessment of the performance of perovskite transistors and phototransistors.
Field-effect transistors (FETs) are key elements in modern electronics and hence are attracting immense scientific and commercial attention. The recent emergence of metal halide perovskite materials and their tremendous success in the field of photovoltaics have triggered the exploration of their application in other (opto)electronic devices, including FETs and phototransistors. In this review, the current status of the field is discussed, the challenges are highlighted, and an outlook for the future perspectives of perovskite FETs is provided. First, attention is drawn to the device physics and the fundamental processes that influence these devices, including the role of ion migration and defects, effects of temperature, light, and measurement conditions. Next, the performance of perovskite transistors and phototransistors reported to date are surveyed and critically assessed. Finally, the key challenges that impede perovskite transistor progress are outlined and discussed. The insights gained from the study of other perovskite optoelectronic devices may be adopted to address these challenges and advance this exciting field of research closer to the industrial application are examined.

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