4.8 Article

Adhesion-Induced Instability Regulates Contact Mechanics of Soft Thin Elastic Films

Journal

ACS APPLIED MATERIALS & INTERFACES
Volume 13, Issue 18, Pages 21994-21999

Publisher

AMER CHEMICAL SOC
DOI: 10.1021/acsami.1c03047

Keywords

soft material interface; contact mechanics; adhesive instability; thin films; indentation

Funding

  1. National Natural Science Foundation of China [12025207, 11872357]
  2. Fundamental Research Funds for the Central Universities
  3. Strategic Priority Research Program of the Chinese Academy of Sciences [XDB22040403]
  4. University of Science and Technology of China Center for Micro and Nanoscale Research and Fabrication

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This study reveals the possibility of fingering instability and inner cavitation during the loading-unloading process of a soft thin elastic film being indented with a spherical indenter. Adhesion-induced instability can enhance the material's resistance to deformation, thus increasing contact force.
Adhesive contact of soft materials plays an essential role in flexible electronics, soft robots, and biological systems. Classical contact mechanics theories assume that the contact region between a spherical indenter and a flat surface is circular. In this paper, however, we show that fingering instability and inner cavitation may appear and disappear during the loading-unloading process when a soft thin elastic film is indented with a spherical indenter. We further demonstrate that this adhesion-induced instability can enhance the resistance to deformation and thus significantly increase contact force. Finally, we find an important dimensionless number, defined as the ratio of adhesion energy to elastic energy, and thus reveal that the competition between adhesion energy and elastic energy yields the critical condition for adhesion-induced instability. Thus, our findings bridge the gap between contact mechanics and interfacial instabilities of soft materials and may have many important implications for the applications of soft materials.

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