4.8 Article

Progress and perspectives of 2D materials as anodes for potassium-ion batteries

Journal

ENERGY STORAGE MATERIALS
Volume 38, Issue -, Pages 354-378

Publisher

ELSEVIER
DOI: 10.1016/j.ensm.2021.03.007

Keywords

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Funding

  1. National Key Research and Development Program of China [2018YFB1502103, 2018YFB1502105]
  2. National Natural Science Foundation of China [U20A20237, 51863005, 51671062, 51871065, 51971068]
  3. Scientific Research and Technology Development Program of Guangxi [AA19182014, AD17195073, AA17202030-1]
  4. Guangxi Bagui Scholar Foundation
  5. Guangxi Collaborative Innovation Centre of Structure
  6. Property for New Energy and Materials, Guangxi Advanced Functional Materials Foundation, and Application Talents Small Highlands
  7. Chinesisch-Deutsche Kooperationsgruppe [GZ1528]

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Researchers are increasingly interested in the development of rechargeable batteries using potassium instead of lithium as the charge carrier, as this technology is considered a promising choice for large-scale energy storage. However, research on potassium ion batteries (PIBs) is still in its early stages, facing various challenges, including the need to find a suitable anode material. Two-dimensional materials show great potential in battery applications due to their unique properties.
The development of rechargeable batteries using potassium instead of lithium as charge carrier is being studied with increasing interest. Potassium ion batteries (PIBs) are considered as a promising technology for large-scale energy storage, due to the advantages of using K, such as earth-abundance and cost effectiveness. Nevertheless, research on PIBs is still in its infancy and faces numerous challenges. Among these, a primary one is to identify a suitable anode material which has multiple properties, specifically high specific capacity, long-term life cycle, fast charging, low-cost, environmental friendliness and meets safety standards. Two-dimensional (2D) materials show great potential in battery applications due to their properties, such as large specific area, enlarged interlayer distance and surface modifiability. We review the state of the art on the synthesis and application of 2D materials in PIBs, including graphene, MXenes, transition-metal dichalcogenide materials, graphene-analogous materials and porous polymer materials. The electrochemical characteristics of different materials and K+ storage mechanisms are presented, and current challenges as well as some promising approaches for the future development of PIBs are also proposed.

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