Compensating for artifacts in scanning near-field optical microscopy due to electrostatics

Nanotechnology and modern materials science demand reliable local probing techniques on the nanoscopic length scale. Most commonly, scanning probe microscopy methods are applied in numerous variants and shades, for probing the different sample properties. Scattering scanning near-field optical microscopy (s-SNOM), in particular, is sensitive to the local optical response of a sample, by scattering light off an atomic force microscopy (AFM) tip, yielding a wavelength-independent lateral resolution in the order of similar to 10 nm. However, local electric potential variations on the sample surface may severely affect the probe-sample interaction, thereby introducing artifacts into both the optical near-field signal and the AFM topography. On the other hand, Kelvin-probe force microscopy (KPFM) is capable of both probing and compensating such local electric potentials by applying a combination of ac and dc-voltages to the AFM tip. Here, we propose to combine s-SNOM with KPFM in order to compensate for undesirable electrostatic interaction, enabling the in situ probing of local electric potentials along with pristine optical responses and topography of sample surfaces. We demonstrate the suitability of this method for different types of materials, namely, metals (Au), semiconductors (Si), dielectrics (SiO2), and ferroelectrics (BaTiO3), by exploring the influence of charges in the systems as well as the capability of KPFM to compensate for the resulting electric force interactions.

Automated summary

Nanotechnology and modern materials science require reliable local probing techniques at the nanoscale. Different scanning probe microscopy methods, including scattering scanning near-field optical microscopy (s-SNOM) and Kelvin-probe force microscopy (KPFM), can be combined to compensate for undesirable electrostatic interactions and enable in situ probing of local electric potentials on sample surfaces.