4.7 Article

TROPOMI NO2 in the United States: A Detailed Look at the Annual Averages, Weekly Cycles, Effects of Temperature, and Correlation With Surface NO2 Concentrations

Journal

EARTHS FUTURE
Volume 9, Issue 4, Pages -

Publisher

AMER GEOPHYSICAL UNION
DOI: 10.1029/2020EF001665

Keywords

NO2 exposures; NO2 vs; PM2; 5; NOx emissions; remote sensing; TROPOMI NO2; weekday‐ weekend effect

Funding

  1. Department of Energy, Office of Fossil Energy
  2. Health and Air Quality (HAQ) grant [80NSSC19K0193]
  3. Atmospheric Composition Modeling and Analysis Program [80NSSC17K0280, 80NSSC19K0946]
  4. Argonne, a US Department of Energy Office of Science laboratory [DE-AC02-06CH11357]

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This study explores the capabilities of the Tropospheric Monitoring Instrument (TROPOMI) in observing the spatial and temporal patterns of NO2 pollution in the continental United States, revealing its ability to differentiate sources in urban and rural areas, variations between weekdays and weekends, and correlations with temperature. The study also demonstrates a strong correlation between TROPOMI NO2 satellite data and surface-level concentrations, making it advantageous for policymakers and public health officials needing high-resolution and timely information for regulatory purposes.
Observing the spatial heterogeneities of NO2 air pollution is an important first step in quantifying NOX emissions and exposures. This study investigates the capabilities of the Tropospheric Monitoring Instrument (TROPOMI) in observing the spatial and temporal patterns of NO2 pollution in the continental United States. The unprecedented sensitivity of the sensor can differentiate the fine-scale spatial heterogeneities in urban areas, such as emissions related to airport/shipping operations and high traffic, and the relatively small emission sources in rural areas, such as power plants and mining operations. We then examine NO2 columns by day-of-the-week and find that Saturday and Sunday concentrations are 16% and 24% lower respectively, than during weekdays. We also analyze the correlation of daily maximum 2-m temperatures and NO2 column amounts and find that NO2 is larger on the hottest days (>32 degrees C) as compared to warm days (26 degrees C-32 degrees C), which is in contrast to a general decrease in NO2 with increasing temperature at moderate temperatures. Finally, we demonstrate that a linear regression fit of 2019 annual TROPOMI NO2 data to annual surface-level concentrations yields relatively strong correlation (R-2 = 0.66). These new developments make TROPOMI NO2 satellite data advantageous for policymakers and public health officials, who request information at high spatial resolution and short timescales, in order to assess, devise, and evaluate regulations.

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