4.6 Article

Transmitting Surface Plasmon Polaritons across Nanometer-Sized Gaps by Optical near-Field Coupling

Journal

ACS PHOTONICS
Volume 8, Issue 3, Pages 832-840

Publisher

AMER CHEMICAL SOC
DOI: 10.1021/acsphotonics.0c01797

Keywords

Surface Plasmon Polaritons; Light Confinement; Helium Ion Microscopy; Nanofocusing; Sketch and Peel; Near-Field Coupling

Funding

  1. Deutsche Forschungsgemeinschaft [SPP1839, SPP1840]
  2. Korea Foundation for International Cooperation of Science and Technology (Global Research Laboratory project) [K20815000003]
  3. BMBF

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Metallic nanostructures can transport electromagnetic fields as surface plasmon polaritons, enabling efficient light-matter coupling on the nanoscale. Experimental demonstration of this phenomenon using bow-tie antennas with curved line gratings highlights the importance of optical near-field coupling in achieving high transmission efficiency.
Metallic nanostructures can transport electromagnetic fields in the form of surface plasmon polariton (SPP) excitations, focus them into nanometric spots, and transfer them to nearby nanostructures by near-field coupling. This provides a basic functionality for designing new plasmonic devices that can greatly enhance light-matter coupling and facilitate ultrafast and efficient all-optical switching on the nanoscale. Here, we study a prototypical device geometry, a bow-tie antenna equipped with curved line gratings, for the efficient coupling of light into and across the antenna nanogap. We experimentally demonstrate the spectrally broadband launching and propagation of SPP waves over more than 10 mu m on one arm of the antenna, their focusing into and transmission across the gap being studied by the plasmon outcoupling on the other arm. A substantial increase in the coupling efficiency for antennas with gap widths below 20 nm proves that the optical near-field coupling between the two antenna arms dominates the gap transmission. We find overall transmission efficiencies for nanofocusing, gap transmission, and plasmon outcoupling of up to 4%. A finite-difference time-domain simulation supports our experimental findings. This makes such bow-tie couplers an interesting platform for sensitively probing near-field coupling to single quantum emitters and for the ultrafast switching of light by light on the nanoscale.

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