Spontaneously coherent orbital coupling of counterrotating exciton polaritons in annular perovskite microcavities

Exciton-polariton condensation is regarded as a spontaneous macroscopic quantum phenomenon with phase ordering and collective coherence. By engineering artificial annular potential landscapes in halide perovskite semiconductor microcavities, we experimentally and theoretically demonstrate the room-temperature spontaneous formation of a coherent superposition of exciton-polariton orbital states with symmetric petal-shaped patterns in real space, resulting from symmetry breaking due to the anisotropic effective potential of the birefringent perovskite crystals. The lobe numbers of such petal-shaped polariton condensates can be precisely controlled by tuning the annular potential geometry. These petal-shaped condensates form in multiple orbital states, carrying locked alternating pi phase shifts and vortex-antivortex superposition cores, arising from the coupling of counterrotating exciton-polaritons in the confined circular waveguide. Our geometrically patterned microcavity exhibits promise for realizing room-temperature topological polaritonic devices and optical polaritonic switches based on periodic annular potentials.

Automated summary

Exciton-polariton condensation has been experimentally and theoretically demonstrated to form coherent superposition of exciton-polariton orbital states in halide perovskite semiconductor microcavities at room temperature by engineering artificial annular potential landscapes. The petal-shaped polariton condensates can be precisely controlled by tuning the annular potential geometry, and exhibit locked alternating pi phase shifts and vortex-antivortex superposition cores. This study opens up possibilities for topological polaritonic devices and optical polaritonic switches based on periodic annular potentials in geometrically patterned microcavities.