4.8 Article

High-frequency rectifiers based on type-II Dirac fermions

Journal

NATURE COMMUNICATIONS
Volume 12, Issue 1, Pages -

Publisher

NATURE RESEARCH
DOI: 10.1038/s41467-021-21906-w

Keywords

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Funding

  1. State Key Program for Basic Research of China [2017YFA0305500, 2018YFA0306204]
  2. National Natural Science Foundation of China [61521005, 61875217, 91850208]
  3. STCSM Grants [1859078100, 19590780100]
  4. Science Education and Research Board (SERB)
  5. Department of Science and Technology (DST) of the government of India
  6. Analytical Instrumentation Center [SPST-AIC10112914]
  7. Soft Matter Nanofab [SPST-SMN180827]
  8. Quantum Device Lab, Shanghai Tech University
  9. ICTP Programme for Training and Research in Italian Laboratories, Trieste, Italy
  10. State Key Laboratory for Modification of Chemical Fibers and Polymer Materials, Donghua University [KF1809]

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Researchers have developed homogeneous rectifiers based on topological semimetal-NiTe2, converting high-frequency electromagnetic energy into direct current with high efficiency. These devices demonstrate room-temperature photosensitivity and performance, validating the potential of controlling nonequilibrium topological states for high-frequency operations and sensitive sensing applications.
The advent of topological semimetals enables the exploitation of symmetry-protected topological phenomena and quantized transport. Here, we present homogeneous rectifiers, converting high-frequency electromagnetic energy into direct current, based on low-energy Dirac fermions of topological semimetal-NiTe2, with state-of-the-art efficiency already in the first implementation. Explicitly, these devices display room-temperature photosensitivity as high as 251mAW(-1) at 0.3THz in an unbiased mode, with a photocurrent anisotropy ratio of 22, originating from the interplay between the spin-polarized surface and bulk states. Device performances in terms of broadband operation, high dynamic range, as well as their high sensitivity, validate the immense potential and unique advantages associated to the control of nonequilibrium gapless topological states via built-in electric field, electromagnetic polarization and symmetry breaking in topological semimetals. These findings pave the way for the exploitation of topological phase of matter for high-frequency operations in polarization-sensitive sensing, communications and imaging. High-frequency rectifiers at terahertz regime are pivotal components in modern communication, whereas the drawbacks in semiconductor junctions-based devices inhibit their usages. Here, the authors report electromagnetic rectification with high signal-to-noise ratio driven by chiral Bloch-electrons in type-II Dirac semimetal NiTe2-based device allowing for efficient THz detection.

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