Journal
NATURE MATERIALS
Volume 20, Issue 5, Pages 624-+Publisher
NATURE PORTFOLIO
DOI: 10.1038/s41563-020-00892-2
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Funding
- Excellent Young Scientist Foundation of NSFC [51522301]
- National Natural Science Foundation of China [22075009, 51961130388, 21875010, 51103004, 52003011]
- Newton Advanced Fellowship [NAF\R1\191235]
- Beijing Natural Science Foundation [JQ19006]
- National Postdoctoral Programme for Innovative Talents [BX20200038]
- China Postdoctoral Science Foundation [2019M660387]
- 111 Project [B14009]
- Postdoctoral Research Program on Innovative Practice in Jiangmen and Excellent Sino-Foreign Young Scientist Exchange Program of CAST
- Air Force Office of Scientific Research [FA9550-18-1-0510]
- Robert A. Welch Foundation [AT-0029]
- National Science Award [CMMI1636306]
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The study used covalent and pi-pi inter-platelet bridging to permanently freeze the stretch-induced alignment of graphene sheets, increasing the isotropic in-plane sheet strength to 1.55 GPa, while maintaining a high Young's modulus, electrical conductivity and weight-normalized shielding efficiency. The graphene sheets fabricated at near room temperature are scalable and can be easily bonded together using a commercial resin without significantly decreasing performance.
Abstracct Efforts to obtain high-strength graphene sheets by near-room-temperature assembly have been frustrated by the misalignment of graphene layers, which degrades mechanical properties. While in-plane stretching can decrease this misalignment, it reappears when releasing the stretch. Here we use covalent and pi-pi inter-platelet bridging to permanently freeze stretch-induced alignment of graphene sheets, and thereby increase isotropic in-plane sheet strength to 1.55 GPa, in combination with a high Young's modulus, electrical conductivity and weight-normalized shielding efficiency. Moreover, the stretch-bridged graphene sheets are scalable and can be easily bonded together using a commercial resin without appreciably decreasing the performance, which establishes the potential for practical applications. Stretch-induced alignment of graphene sheets is frozen by sequential covalent and pi-pi bridging, leading to high in-plane isotropic strength of 1.55 GPa. The graphene sheets are fabricated at near room temperature and are scalable.
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