4.6 Article

In Situ Tuning Underwater Bubble Movement on Slippery Lubricant-Infused Anisotropic Microgrooved Surface by Unidirectional Mechanical Strain

Journal

LANGMUIR
Volume 37, Issue 6, Pages 2140-2145

Publisher

AMER CHEMICAL SOC
DOI: 10.1021/acs.langmuir.0c03330

Keywords

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Funding

  1. National Natural Science Foundation of China [51805508, 51875152, 51975174]
  2. China Postdoctoral Science Foundation [2020T130632]

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Research focuses on designing and fabricating functional interfaces to control the movement behavior of underwater gas bubbles. A slippery lubricant-infused anisotropic microgrooved surface (SLI-AMGS) was successfully fabricated using femtosecond laser direct writing technology, allowing for reversible switching between underwater bubble sliding and pinning. By changing mechanical tensile strain, real-time dynamic modulation of underwater bubbles was demonstrated in different acid-based environments, showing potential applications in various fields such as underwater bubble microfluidics and microbubble robots.
Numerous studies have focused on designing and fabricating functional interfaces that control movement behavior of underwater gas bubbles, which are ubiquitous in a variety of natural and industrial settings. Nevertheless, developing surfaces with in situ tunable bubble movement remain elusive because of current complicated tuning strategies on the specific materials. Inspired by natural pitcher plant and rice leaves, here we report a kind of slippery lubricant-infused anisotropic microgrooved surface (SLI-AMGS) fabricated by femtosecond laser direct writing technology and realize the in situ reversible switching between underwater bubble sliding and pinning by unidirectional mechanical tensile strain. Different experimental parameters including lubricant oil film thickness, bubble volumes and laser power have been researched to manifest the relationship with bubble sliding behaviors. The underlying mechanism of in situ reversible switching mainly lies on the decrease of the lubricant oil film thickness during the process of mechanical stretching in which the uniform and stable oil film layer becomes uneven. This uneven lubricant oil film results in an extraordinary increase of contact angle hysteresis and resistance. At last, we demonstrate a real-time dynamic modulation of the underwater bubble on the SLI-AMGS with a changing mechanical tensile strain for several repeatable times in different acid-based environments. Our work manifests great potential applications in widespread fields including underwater bubble microfluidics and microbubble robots.

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