4.7 Article

Genesis of electric field assisted microparticle assemblage in a dielectric fluid

Journal

JOURNAL OF FLUID MECHANICS
Volume 915, Issue -, Pages -

Publisher

CAMBRIDGE UNIV PRESS
DOI: 10.1017/jfm.2021.22

Keywords

multiphase and particle-laden flows; MHD and electrohydrodynamics

Funding

  1. DST SERB [EMR/2016/001824, 5(9)/2012-NANO]
  2. Government of India

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The oscillatory motions of charged particles in a liquid medium and the aggregation process in multi-particle systems are influenced by the properties of the surrounding fluid. Different sized particles exhibit elastic or inelastic collisions, with equal-sized particles showing synchronized motions and unequal-sized particles showing non-uniform motions. Additionally, charge reversal and the presence of counter-rotating vortices surrounding charged particles have been observed in multi-particle systems.
Oscillatory motions of charged particles inside a liquid medium have been explored under the influence of an electric field emulating field-induced particle-laden fluid flows. The properties of the surrounding fluid are found to play key roles in the kinetics of such a particle aggregation process. While the weakly conducting or insulating liquids promote high-frequency oscillations of charged particles followed by a quick assemblage, the viscosity and relative permittivity of the liquid play significant roles in modulating the time scale. In fact, the origin of such motions in a multi-particle system is very similar to a system with a single charged particle wherein the particle gathers charge from one of the electrodes before moving towards the other of opposite polarity. Interestingly, in the multi-particle system, an unprecedented charge reversal is observed wherein a charged particle reverses its direction of motion after colliding with another particle of opposite polarity. Experiments together with simulations further reveal that, while the equal-sized particles undergo an electric field driven 'elastic' collision and show synchronized motions with nearly similar speeds of approach and separation, the motions of unequal-sized particles are rather non-uniform after undergoing an 'inelastic' collision. Importantly, the simulations with two-particle systems uncover the presence of counter-rotating vortices surrounding the charged particles. The results reported not only usher the genesis of the chain-like assemblage in the multi-particle systems but also open up the possibility of the generation of on-demand power-law liquid properties through 'chaining' or 'layering' of the charged particles.

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