4.6 Article

Universal Criterion for Critical Motion of Droplets Adhered on Surfaces with Different Wettability in Laminar Flow

Journal

INDUSTRIAL & ENGINEERING CHEMISTRY RESEARCH
Volume 60, Issue 8, Pages 3397-3410

Publisher

AMER CHEMICAL SOC
DOI: 10.1021/acs.iecr.0c05957

Keywords

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Funding

  1. National Natural Science Foundation of China [52004141, 51774312]
  2. China Postdoctoral Science Foundation [2020M682185]
  3. Qingdao Applied Research Project [62420070311122]
  4. Shandong Provincial key laboratory of Oil & Gas Storage and Transportation Safety
  5. Qingdao Key Laboratory of Circle Sea Oil & Gas Storage and Transportation Technology

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This study established a universal criterion and mathematical model describing the initial motion of oil droplets on surfaces with different wettability immersed in water, revealing the movement mechanism of oil droplets and investigating the coupling effects of droplet height, surface properties, and water flow velocity on droplet motion behavior. The research obtained the critical shear water flow velocity required for the initial movement of oil droplets from different surfaces, which is of great scientific significance for improving theoretical systems of multiphase separation and guiding the design and optimization of surface properties and flow field velocity.
The initial motion of micro-oil droplets on substrates immersed in water is of great significance to study droplet motion. Here, microscopic experiments and mechanism analysis are used to establish a universal criterion and a mathematical model describing the critical conditions for the initial motion of droplets adhered on surfaces with different wettability in the laminar flow. We demonstrate a surface modification technique and analysis method in a microtest. Based on the force's analysis on the three-phase contact points of two-dimensional oil droplets on the surfaces, the movement mechanism is also obtained when the oil droplets start to move. In addition, this work focuses on the coupling effects of oil droplet's height, surface properties, and water flow velocity on the initial motion behaviors of oil droplets and obtains the critical shear water flow velocity required for the critical movement of oil droplets from different surfaces. We achieve a universal criterion and model for different application scenarios, which are of great scientific significance to improve theoretical systems of multiphase separation and guide the design and optimization of surface properties and flow field velocity.

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