4.7 Article

Experimental study of the influence of hydrogen as a fuel additive on the formation of soot precursors and particles in atmospheric laminar premixed flames of methane

Journal

FUEL
Volume 287, Issue -, Pages -

Publisher

ELSEVIER SCI LTD
DOI: 10.1016/j.fuel.2020.119517

Keywords

Hydrogen; Methane; Premixed flame; PAHs; Soot nucleation; Soot

Funding

  1. Agence Nationale de la Recherche through the LABEX CAPPA [ANR-11-LABX-0005]
  2. R'egion Hauts-de-France
  3. Minist`ere de l'Enseignement Sup'erieur et de la Recherche (CPER Climibio)
  4. European Fund for Regional Economic Development

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Experimental investigation on methane premixed flames with and without hydrogen showed that the introduction of hydrogen has insignificant impact on the maximum mole fractions of small species in the flame.
We report here the experimental investigation of lightly sooting methane premixed flames with and without hydrogen. Two different approaches were considered to introduce hydrogen in the methane flame, either by keeping the total gas flow rate constant or not. Speciation data were obtained using a set of analytical tools including Gas Chromatography, Fourier-Transform Infrared Spectroscopy, Jet-Cooled Laser-Induced Fluorescence, Laser-induced Incandescence coupled with Cavity Ring-Down Spectroscopy. The results include mole fraction profiles of gaseous species (C-0-C-16) and soot volume fraction (f(v)) measured in all studied flames. These results demonstrate that the introduction of hydrogen to the flame insignificantly impacts the maximum mole fractions of small species (

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