4.7 Article

Coupled with EDDS and approaching anode technique enhanced electrokinetic remediation removal heavy metal from sludge

Journal

ENVIRONMENTAL POLLUTION
Volume 272, Issue -, Pages -

Publisher

ELSEVIER SCI LTD
DOI: 10.1016/j.envpol.2020.115975

Keywords

Sludge; Heavy metal; Ethylenediamine disuccinic acid (EDDS); Electrokinetic remediation; Approaching anode electrokinetic technique

Funding

  1. Talent Introduction Funds of the Sichuan University of Science and Engineering [2020RC23]
  2. National Natural Science Foundation of China [51978576]
  3. Sichuan Province Key Technology Support [2019YFN0027]

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In this study, a novel technology was applied to remove heavy metals from sludge, with the coupled EDDS and AA-EK technique showing enhanced efficiency. The results indicated that the technique led to increased electric current and predominant heavy metal removal, demonstrating its effectiveness in electrokinetic remediation.
In this work, the novel technology was used to remove heavy metal from sludge. The coupled with biodegradable ethylenediamine disuccinic acid (EDDS) and approaching anode electrokinetic (AA-EK) technique was used to enhance heavy metal removing from sludge. Electric current, sludge and electrolyte characteristics, heavy metal removal efficiency and residual content distribution, and heavy metal fractions percentage of variation were evaluated during the electrokinetic remediation process. Results demonstrated that the coupled with EDDS and AA-EK technique obtain a predominant heavy metal removal efficiency, and promote electric current increasing during the enhanced electrokinetic remediation process. The catholyte electrical conductivity was higher than the anolyte, and electrical conductivity of near the cathode sludge achieved a higher value than anode sludge during the coupled with EDDS and AA-EK remediation process. AA-EK technique can produce a great number of Hthorn, which caused the sludge acidification and pH decrease. Cu, Zn, Cr, Pb, Ni and Mn obtain the highest extraction efficiency after the coupled with EDDS and AA-EK remediation, which were 52.2 +/- 2.57%, 56.8 +/- 3.62%, 60.4 +/- 3.62%, 47.2 +/- 2.35%, 53.0 +/- 3.48%, 54.2 +/- 3.43%, respectively. Also, heavy metal fractions analysis demonstrated that the oxidizable fraction percentage decreased slowly after the coupled with EDDS and AA-EK remediation. (C) 2020 Elsevier Ltd. All rights reserved.

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