Journal
CHEMICAL ENGINEERING JOURNAL
Volume 417, Issue -, Pages -Publisher
ELSEVIER SCIENCE SA
DOI: 10.1016/j.cej.2021.129325
Keywords
Anaerobic osmosis membrane bioreactor (AnOMBR); Waste activated sludge; Dissolved methane; Water recovery; Biogas upgrading
Categories
Funding
- China National Key Project of Science and Technology Major Science and Technology Program for Water Pollution Control and Treatment [2018ZX07601001]
- Fundamental Research Funds for the Central Universities [DUT20LAB101]
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Anaerobic osmotic membrane bioreactors (AnOMBRs) have great potential for water and energy recovery, with performance being influenced by draw solution (DS) concentrations and temperatures. Optimal results for treating low-strength waste activated sludge were achieved at a DS concentration of 0.75 M, with higher concentrations causing membrane fouling and decreased methanogen activity. The study showed that specific methanogenic activity was suppressed under higher DS concentrations, controlling the performance of AnOMBR to some extent.
Anaerobic osmotic membrane bioreactors (AnOMBRs) have a great potential for water and energy recovery, but performance of AnOMBRs regulated by draw solution (DS) concentrations (0.5 M - 1.5 M) and temperatures (15 degrees C - 35 degrees C) should be further enhanced. The results showed that the highest water production capacity of AnOMBR treating low-strength waste activated sludge was achieved under DS concentration of 0.75 M. When DS concentration exceeded this critical value, aggravated membrane fouling and cake-enhanced concentration polarization caused a negative contribution for net driving force maintenance of FO progress. More importantly, specific methanogenic activity of acetoclastic methanogens was suppressed under higher DS concentrations which further suggested that performance of AnOMBR was controlled by DS concentration to some extent. Under the critical DS concentration, removal of soluble chemical oxygen demand was above 90% during 60 days operation of AnOMBR. Dissolved methane in the bulk solution were not oversaturated at a ratio of 0.66, 0.48 and 0.17 and energy recovery of 2.0 kWh/m(3), 3.1 kWh/m(3) and 4.2 kWh/m(3) was achieved at 15 degrees C, 25 degrees C and 35 degrees C, respectively. When AnOMBR was integrated with a microbial electrolysis cell (AnOMBR-MEC), CH4 component of AnOMBR-MEC was 97% and energy recovery reached at 5.1 kWh/m(3) at 25. due to synergetic effect of electrochemical CO2 reduction by cathode and bio-conversion of produced formate. This work demonstrated that the optimal condition was DS concentration of 0.75 M under 25 degrees C for water (energy) recovery enhancement and biogas upgrading for AnOMBR-MEC simultaneously.
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