4.7 Article

Enhanced wood-derived photothermal evaporation system by in-situ incorporated lignin carbon quantum dots

Journal

CHEMICAL ENGINEERING JOURNAL
Volume 405, Issue -, Pages -

Publisher

ELSEVIER SCIENCE SA
DOI: 10.1016/j.cej.2020.126703

Keywords

Photothermal evaporation; Seawater desalination; Simulation and numerical modelling; Carbon quantum dots; Wood-based resources utilization

Funding

  1. National Natural Science Foundation of China [31770605, 31822008]
  2. Outstanding Youth Foundation of Heilongjiang [JC2018006]

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The novel green photothermal evaporation system shows high efficiency and stability, with economic and ecological advantages. Through simulation and numerical modeling, the key factors affecting water transportation and evaporation processes were analyzed.
Photothermal evaporation and desalination via renewable solar energy has promising potential to alleviate freshwater scarcity. However, recent reported systems usually lack sufficient environmental compatibility, ecological security, and energy-saving concern. Here, a novel and green photothermal evaporation system with ecological and economic advantages was designed. An evaporation performance of 1.18 kg.m(-2) (1.09 kg.m(-2).h(-1)) with up to 79.5% efficiency at one sun illumination (1 kW.m(-2)) was achieved. More importantly, a series of simulation and numerical modelling was synchronously developed to analyze in-depth the main factors that affect water transportation and evaporation processes. The channel size, temperature distribution, and formed gradient were carefully investigated and discussed. Notably, this system exhibited satisfactory repeatability and stability. In addition, only a few photothermal components are required in this system, which will also bring a significant economic merit. Taken together, this work successfully provides new insights into developing a sustainable photothermal evaporation system with ecologically friendly property and satisfactory performance in practical application. Moreover, it also reveals the corresponding water transportation and photothermal evaporation mechanisms, and maximizes the evaporation efficiency.

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