4.8 Article

Diamond-graphite nanocomposite synthesized from multi-walled carbon nanotubes fibers

Journal

CARBON
Volume 172, Issue -, Pages 138-143

Publisher

PERGAMON-ELSEVIER SCIENCE LTD
DOI: 10.1016/j.carbon.2020.10.024

Keywords

Diamond; Graphite; Nanocomposite; Multi-walled carbon nanotubes; Laser heating

Funding

  1. National Natural Science Foundation of China [51822204, 11634004, U1604263, 11804307]
  2. China Postdoctoral Science Foundation [2018M630830, 2019T120631]
  3. Open Project of State Key Laboratory of Superhard Materials (Jilin University) [201702]

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The study introduces a new method for the synthesis of diamond-graphite hybrid nanocomposite from multi-walled carbon nanotubes fibers using laser heating diamond anvil cell, with a combined theory-experiment approach confirming the formation of the hybrid structure. This approach opens up a new avenue for generating new carbon nanocomposites using high pressure techniques and other suitable carbon precursors.
Creation of the hybrid nanostructures with superior properties that combine the advantages of hardest diamond and flexible graphite remains challenging in experiment. Here we report a new strategy for the synthesis of diamond-graphite hybrid nanocomposite from multi-walled carbon nanotubes fibers by laser heating diamond anvil cell. A combined theory experiment approach confirms the formation of diamond-graphite hybrid structure with the coherent interface consisted of covalent bonds between diamond and graphite. This opens an avenue for the synthesis of diamond-graphite hybrid structure, which may be extended to generate new carbon nanocomposites using other suitable carbon precursors by high pressure. (C) 2020 Elsevier Ltd. All rights reserved.

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