4.6 Article

Modulating the transport property of flexible La0.67Ca0.33MnO3 thin film by mechanical bending

Journal

APPLIED PHYSICS LETTERS
Volume 118, Issue 5, Pages -

Publisher

AIP Publishing
DOI: 10.1063/5.0024516

Keywords

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Funding

  1. Natural Science Foundation of China [51702255, 51390472]
  2. National 973 projects of China [2015CB654903, 2015CB654603]
  3. Shaanxi Natural Science Foundation [2019JM-068]
  4. Fundamental Research Funds for the Central Universities

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Research has shown that flexible epitaxial LCMO thin films fabricated on SrTiO3-buffered fluorophlogopite substrates exhibit a metal-to-insulator transition tendency towards lower temperature when subjected to mechanical bending. The transport behavior of the bent LCMO films follows the variable range hopping model in the insulating region, with resistivity increasing as bending curvature radii decrease, making them promising for use as low-temperature mechanical-bending switch devices.
Flexible epitaxial La0.67Ca0.33MnO3 (LCMO) thin films are fabricated on an SrTiO3 buffered (001)-oriented fluorophlogopite substrate. The metal-to-insulator transition tends toward lower temperature when subjected to mechanical bending. Moreover, the transport behavior of the bent LCMO films in the insulating region follows the variable range hopping model and the resistivity increases with the reduction in the bending curvature radii because the applied strain aggravates the distortion of the LCMO crystal structure, decreases the hopping distance, and, hence, impedes the transport of charge carriers. The resistivity change induced by the mechanical bending can go up to 10(4)% at 100K and 10(5)% at 10K. Such a large resistivity change makes the flexible LCMO thin film promising as a mechanical-bending switch device at low temperature.

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