Journal
ANGEWANDTE CHEMIE-INTERNATIONAL EDITION
Volume 60, Issue 18, Pages 9941-9946Publisher
WILEY-V C H VERLAG GMBH
DOI: 10.1002/anie.202100434
Keywords
3D covalent organic frameworks; charge transport; interpenetration; non-planar aromatics; polycyclic aromatic hydrocarbons
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Funding
- Basque Science Foundation for Science (Ikerbasque)
- POLYMAT
- University of the Basque Country [GIU17/054]
- Gobierno de Espana (Ministerio de Ciencia e Innovacion, Plan Estatal de Investigacion Cientifica y Tecnica y de Innovacion)
- Gobierno Vasco (PIBA programme)
- European Research Council (ERC) under the European Union [722951]
- European Union's Horizon 2020 research and innovation programme [664878, 899895]
- Portuguese Foundation for Science and Technology/MCTES [IF/00894/2015, UIDB/50011/2020, UIDP/50011/2020]
- Gobierno Vasco (BERC programme)
- ERDF
- ESF
- European Research Council (ERC) [722951] Funding Source: European Research Council (ERC)
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3D COFs with pcu topology are obtained from distorted polycyclic aromatic hydrocarbons acting as triangular antiprismatic (D-3d) nodes. These 3D COFs exhibit six-fold interpenetration due to interframework pi-stacking, leading to unexpected charge transport properties.
Three-dimensional covalent organic frameworks (3D COFs) with a pcu topology have been obtained from distorted polycyclic aromatic hydrocarbons acting as triangular antiprismatic (D-3d) nodes. Such 3D COFs are six-fold interpenetrated as the result of interframework pi-stacking, which enable charge transport properties that are not expected for 3D COFs.
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