4.8 Article

Omnidirectional Control of Large Electrical Output in a Topological Antiferromagnet

Journal

ADVANCED FUNCTIONAL MATERIALS
Volume 31, Issue 15, Pages -

Publisher

WILEY-V C H VERLAG GMBH
DOI: 10.1002/adfm.202008971

Keywords

anomalous hall effect; anomalous nernst effect; antiferromagnetic spintronics; memory; sensors; topological magnet

Funding

  1. CREST [JPMJCR18T3, JPMJCR15Q5]
  2. JST-Mirai Program [JPMJMI20A1]
  3. Japan Science and Technology Agency
  4. New Energy and Industrial Technology Development Organization (NEDO)
  5. Ministry of Education, Culture, Sports, Science, and Technology of Japan [15H05882, 15H05883]
  6. Program for Advancing Strategic International Networks to Accelerate the Circulation of Talented Researchers from the Japanese Society for the Promotion of Science (JSPS) [R2604]
  7. SHINES, an Energy Frontier Research Center of US Department of Energy [SC0012670]
  8. US Department of Energy, office of Basic Energy Sciences, Division of Materials Sciences and Engineering [DE-FG02-08ER46544]
  9. [DE-SC0009390]
  10. [19H00650]

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Control of magnetization direction is crucial for ferromagnets, but large magnetization can limit directional control. Topological metallic states in antiferromagnets offer strong responses, potentially replacing ferromagnets in magnetic devices.
Control of magnetization direction is essential for the wide application of ferromagnets; it defines the signal size of memory and sensor. However, the magnetization itself causes a dilemma. While its size matters to obtain strong responses upon its reversal, the large magnetization concomitantly suppresses the range of its directional control because of the demagnetizing field. On the other hand, realization of the desired magnetic anisotropy requires careful engineering of crystalline and interfacial effects to overcome the demagnetization barrier. Thus, it would be ideal if one could find alternative magnets that carry no magnetization but strong responses. The discovery of a topological metallic state in the antiferromagnet Mn3Sn is significant; they host a large Berry curvature in momentum space, enabling the observation of disproportionately large transverse responses such as anomalous Hall and Nernst effects, the key functionalities for replacing ferromagnets in the magnetic devices. Here, the experimental realization of omnidirectional control of the large responses in an antiferromagnet is reported. In particular, it is demonstrated that the absence of shape anisotropy enables the omnidirectional control, and lifts the shape constraint in designing the magnetic devices. This work lays the technological foundation for developing simple-structured high-performance devices including multi-level memory and heat flux sensor.

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