Journal
ELECTROCHIMICA ACTA
Volume 222, Issue -, Pages 1650-1659Publisher
PERGAMON-ELSEVIER SCIENCE LTD
DOI: 10.1016/j.electacta.2016.11.155
Keywords
Reduced graphene oxide nanosheets; Cu2O-CuO-RGO; Sandwich structure; Anode materials; Solvothermal
Categories
Funding
- National Natural Science Foundation of China [21471100, 51502177, 21001074]
- Training Foundation for Outstanding Young Teachers in Higher Education Institutions of Guangdong [YQ2015146]
- Natural Science Foundation of Guangdong [2014A030310323]
- Shenzhen Dedicated Funding of Strategic Emerging Industry Development Programme [JCYJ20140418182819158]
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Ternary copper oxides/reduced graphene oxide (Cu2O-CuO-RGO) composites were successfully synthesized in situ by a self-assembly solvothermal method in a water-ethanol mixture and used directly as the anode material for lithium ion batteries. The Cu2O-CuO-RGO composites delivered a reversible capacity of 842.5 mAh g(-1) after 80 cycles at a current density of 100 mA g(-1), and after every 10 cycles at current densities of 100, 200, 500, 1000, 2000, 5000 and 100 mA g(-1), respectively, the specific capacities of the composites were approximately 840, 723, 511, 402, 336, 224, and 703 mAh g(-1), respectively. The improved electrochemical performance of the composites is closely related to its sandwich structure, with multicomponent Cu2O-CuO nanospheres adhering tightly to both sides of RGO nanosheets. This structure could shorten the transport pathways for both electrons and lithium ions, prevent the RGO nanosheets from stacking, enhance the electrical conductivity and accommodate the volume expansion that occurs during prolonged cycling. (C) 2016 Elsevier Ltd. All rights reserved.
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