Journal
RESULTS IN PHYSICS
Volume 19, Issue -, Pages -Publisher
ELSEVIER
DOI: 10.1016/j.rinp.2020.103404
Keywords
SiO2 microsphere; Langmuir-Blodgett technique; Self-assembly; Layer-by-layer transferring technique
Funding
- National Science Foundation of China (NSFC) [11704183, 11974188, 11704184, 51701176]
- NUPTSF [NY219015]
- Double Innovation Project of Jiangsu Province [CZ106SC19010]
- China Postdoctoral Science Foundation [2017M621693]
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We report on a rapid and efficient method to self-assemble high-quality monolayer or multilayers of bare silica microsphere (MS) at the water/air interface. The key to our method is forming an ultra-thin 1-butanol layer achieved by using the mixed suspension with a proper volume ratio of ethanol and 1-butanol (2:1) on the water surface. This ultra-thin 1-butanol can deliver, confine and keep the movement of the SiO2 MS at the air/water interface throughout the self-assembly process, which is of crucial importance for achieving the high-quality of the assembled monolayer. By our method, the hexagonal-close-packed arrangement monolayers of bare SiO2 MS with millimeter-sized (similar to mm) single-domain regions are successfully fabricated for different sizes (diameters: 300, 480, 730, and 990 nm). In addition, the multilayers fabricated by the layer-by-layer transferring technique present the typical photonic bandgap materials feature in the measured transmission spectra. The fabricated high-quality monolayer or multilayers of bare SiO2 MS could be compatible with the high-temperature material grown process and may find potential applications in optoelectmnics and photocatalysis.
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