Journal
ACS CATALYSIS
Volume 11, Issue 2, Pages 967-984Publisher
AMER CHEMICAL SOC
DOI: 10.1021/acscatal.0c04618
Keywords
Cu-promoted inert C(sp(3))-H functionalization; C(sp(3))-C bond formation; C(sp(3))-N bond formation; C(sp(3))-O/S bond formation; C(sp(3))-X bond formation
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Funding
- Recruitment Program of Global Experts (1000 Talents Plan)
- Gansu Province Science Foundation for Distinguished Young Scholars [20JR5RA304]
- Fundamental Research Funds for the Central Universities [lzujbky-2019-ct08]
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This article reviews the main progress of copper-promoted inert C(sp(3))-H functionalization in establishing different types of bonds, presenting reaction characteristics, proposed mechanisms, and future development trends in this field.
Copper-promoted inert C(sp(3))-H functionalization has gradually been developed as a nascent tool to establish categories of bonds, including C(sp(3))-C, C(sp(3))-N, C(sp(3))-O/S, and C(sp(3))-X bonds. However, there have been no reviews summarizing the latest advances in this domain. Herein, we review the main progress of copper-promoted inert C(sp(3))-H functionalization, covering the literature up to 2020 and classifying the works by the types of bonds formed. Reaction characteristics and proposed mechanisms of nearly all examples are presented and, in some cases, are comprehensively compared with those of literature precedents. In addition, an overview of the current development of this field is summarized and the future of this domain is discussed.
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