Journal
ACS CATALYSIS
Volume 11, Issue 1, Pages 248-254Publisher
AMER CHEMICAL SOC
DOI: 10.1021/acscatal.0c04474
Keywords
heteroarene dearomatization; diastereoselective synthesis; heterocycles; copper catalysis; dihydropyridines
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Funding
- Auburn University
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Nucleophilic addition of diborylalkyl reagents to N-alkyl or N-acylpyridinium and related heteroarenium salts has been developed as a key step for the synthesis of nonaromatic nitrogen heterocycles that contain contiguous stereogenic centers. Derivatization of the dihydropyridine products for the synthesis of tetrahydropyridines and piperidines have also been described.
Nucleophilic addition of diborylalkyl reagents to N-alkyl or N-acylpyridinium and related heteroarenium salts has been developed as a key step for the synthesis of nonaromatic nitrogen heterocycles that contain contiguous stereogenic centers. Derivatization of the dihydropyridine products for the synthesis of tetrahydropyridines and piperidines have also been described.
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