Journal
TETRAHEDRON
Volume 82, Issue -, Pages -Publisher
PERGAMON-ELSEVIER SCIENCE LTD
DOI: 10.1016/j.tet.2021.131947
Keywords
Xanthenes; Thioxanthenes; Acridines; Ultraviolet light; Benzylic C(sp(3))-H
Categories
Funding
- National Natural Science Foundation of China [21776260, 21773211, 21773210]
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A mild and efficient system has been discovered for the synthesis of a-aryl carbonyl compounds via oxidation of benzylic C-H to C=O bonds. This oxygenation reaction showed excellent substrate scope and yielded corresponding ketones with good to excellent yields under catalyst- and additive-free conditions at room temperature.
A mild and efficient system has been discovered for the synthesis of a-aryl carbonyl compounds via oxidation of benzylic C-H to C=O bonds. This ultraviolet-light-mediated oxygenation reaction exhibited excellent substrate scope including various xanthenes, thioxanthenes and 9, 10-dihydroacridines and afforded the corresponding ketones with good to excellent yields under catalyst- and additive-free conditions at room temperature. (C) 2021 Elsevier Ltd. All rights reserved.
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