Journal
ORGANIC LETTERS
Volume 22, Issue 23, Pages 9276-9281Publisher
AMER CHEMICAL SOC
DOI: 10.1021/acs.orglett.0c03506
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Funding
- MEXT, Japan [JP26107008, JP19H04573]
- Fusion Emergent Research from the Integrated Research Consortium on Chemical Sciences (IRCCS)
- JSPS KAKENHI [JP18J21819]
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Although many chiral molecules exhibiting circularly polarized luminescence (CPL) have been reported recently, few molecular design guidelines are known for increasing the dissymmetry factor for CPL (g(lum)). We demonstrate that a figure-eight-shaped molecule with D-2 symmetry has excellent chiroptical properties (Phi(f) = 0.08, vertical bar g(lum)vertical bar = 1.5 x 10(-2)), which are attributed to the parallel arrangement of mu and m as well as a good vertical bar mu vertical bar/vertical bar m vertical bar ratio.
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