4.6 Article Proceedings Paper

Growth of Tm:Lu3Al5O12 single crystal fiber from transparent ceramics by laser-heated pedestal method and its spectral properties

Journal

OPTICAL MATERIALS
Volume 111, Issue -, Pages -

Publisher

ELSEVIER
DOI: 10.1016/j.optmat.2020.110674

Keywords

Tm:LuAG; Single crystal fiber; Crystal growth; Judd-Ofelt theory

Funding

  1. Instrument Developing Project of the Chinese Academy of Sciences [YJKYYQ20170019]
  2. International Partnership Program of Chinese Academy of Sciences [121631KYSB20180045]
  3. National Natural Science Foundation of China [51872309, U1832106, 62005302]
  4. Science Foundation for Youth Scholar of State Key Laboratory of High Performance Ceramics and Superfine Microstructures [SKL201904]
  5. Shanghai Science and Technology Commission [18520744300, 20511107400]

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The growth, ion distribution, absorption spectrum, J-O parameters, and emission spectrum of Tm:LuAG single crystal fiber were discussed. Test results showed uniform distribution and stable diameter fluctuation of the fiber, with improved spectral performance for potential use in fiber lasers.
Tm:Lu3Al5O12 (Tm:LuAG) single crystal fiber (SCF) with a diameter of 0.6 mm and a length of 140 mm was grown from transparent ceramics by laser-heated pedestal growth (LHPG) method. The growth, Tm3+ ion distribution, absorption spectrum, Judd-Ofelt (J-O)parameter and emission spectrum of SCF are discussed in detail. The test results show that the diameter fluctuation of the SCF is less than 2% and the Tm3+ ion distribution is relatively uniform. J-O theory was applied to analyze the absorption spectrum. With the J-O intensity parameters Omega(t(t=2,4,6)), the emission probabilities, fluorescence branching ratios and radiative lifetimes for the Tm:LuAG SCF and transparent ceramic were all calculated. The stimulated emission cross-section of the(3)F(4)-> H-3(6) transition was obtained by using the Fuchtbauer-Ladenburg (F-L) method. After comparison, it is found that the spectral performance of Tm:LuAG SCF has been improved to a certain extent on the basis of transparent ceramics. It has the potential to be applied to fiber lasers.

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