4.6 Article

Single-walled carbon nanotube membranes as non-reflective substrates for nanophotonic applications

Journal

NANOTECHNOLOGY
Volume 32, Issue 9, Pages -

Publisher

IOP PUBLISHING LTD
DOI: 10.1088/1361-6528/abcacc

Keywords

carbon nanotube; free-standing thin films; scattering spectroscopy; Mie resonances; nanoparticle imaging

Funding

  1. Russian Foundation for Basic Research [18-32-20217]
  2. Ministry of Education and Science of the Russian Federation [14.W03.31.0008, 0679-2020-0007, FZSR-2020-0007, 075-03-2020-097/1]
  3. MSU Quantum Technology Center
  4. Russian Science Foundation [18-72-00247]
  5. Russian Foundation for Basis Research [18-29-20032]
  6. Russian Science Foundation [18-72-00247] Funding Source: Russian Science Foundation

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It is demonstrated that single-walled carbon nanotube (SWCNT) membranes can enhance visualization and study of individual nanoparticles, showing significant improvement in optical contrast. The high transparency, low reflectance, and thinness of SWCNT membranes offer various potential applications in nanophotonics, bioimaging, and synchrotron radiation studies.
We demonstrate that single-walled carbon nanotube (SWCNT) membranes can be successfully utilized as nanometer-thick substrates for enhanced visualization and facilitated study of individual nanoparticles. As model objects, we transfer optically resonant 200 nm silicon nanoparticles onto pristine and ethanol-densified SWCNT membranes by the femtosecond laser printing method. We image nanoparticles by scanning electron and bright-field optical microscopy, and characterize by linear and Raman scattering spectroscopy. The use of a pristine SWCNT membrane allows to achieve an order-of-magnitude enhancement of the optical contrast of the nanoparticle bright field image over the results shown in the case of the glass substrate use. The observed optical contrast enhancement is in agreement with the spectrophotometric measurements showing an extremely low specular reflectance of the pristine membrane (<= 0.1%). Owing to the high transparency, negligibly small reflectance and thickness, SWCNT membranes offer a variety of perspective applications in nanophotonics, bioimaging and synchrotron radiation studies.

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