4.6 Article

Combined effects of surface plasmon coupling and Forster resonance energy transfer on the light color conversion behaviors of colloidal quantum dots on an InGaN/GaN quantum-well nanodisk structure

Journal

NANOTECHNOLOGY
Volume 32, Issue 13, Pages -

Publisher

IOP Publishing Ltd
DOI: 10.1088/1361-6528/abd05e

Keywords

surface plasmon coupling; Forster resonance energy transfer; quantum dot; Ag nanoparticle; color conversion

Funding

  1. Ministry of Science and Technology, Taiwan, The Republic of China [MOST 109-2221-E-002-194, MOST 108-2221-E-002-160, MOST 107-2923-M-002-005-MY3]
  2. US Air Force Office of Scientific Research [AOARD-17IOA087]

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By forming nanodisk structures on a blue-emitting InGaN/GaN quantum-well template, the efficiency of blue-to-red color conversion can be enhanced. A larger nanodisk height leads to more quantum wells exposed on the sidewall, resulting in higher color conversion efficiency. The strong FRET process and SP coupling effects can enhance the efficiency of blue-to-red color conversion.
By forming nanodisk (ND) structures on a blue-emitting InGaN/GaN quantum-well (QW) template, the QWs become close to the red-emitting quantum dots (QDs) and Ag nanoparticles (NPs) attached onto the sidewalls of the NDs such that Forster resonance energy transfer (FRET) and surface plasmon (SP) coupling can occur to enhance the efficiency of blue-to-red color conversion. With a larger ND height, more QWs are exposed to open air on the sidewall for more QD/Ag NP attachment through QD self-assembly and Ag NP drop casting such that the FRET and SP coupling effects, and hence the color conversion efficiency can be enhanced. A stronger FRET process leads to a longer QD photoluminescence (PL) decay time and a shorter QW PL decay time. It is shown that SP coupling can enhance the FRET efficiency.

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