4.8 Article

Discretely-supported nanoimprint lithography for patterning the high-spatial-frequency stepped surface

Journal

NANO RESEARCH
Volume 14, Issue 8, Pages 2606-2612

Publisher

TSINGHUA UNIV PRESS
DOI: 10.1007/s12274-020-3261-3

Keywords

nanoimprint lithography; non-planar surface; discretely-supported template; nanopatterning; semiconductor light emitting devices

Funding

  1. National Key R&D Program of China [2017YFB1102900]
  2. Natural Science Foundation of China [51805422]
  3. China Postdoctoral Science Foundation [2019M653592]
  4. Basic Research Program of Natural Science of Shaanxi Province of China [2019JLM-5]

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The study introduces a discretely-supported nanoimprint lithography (NIL) technique to address the challenge of nano-patterning on non-planar surfaces, successfully fabricating nanostructures on LED chips and increasing optical output power by more than 40%. This innovation could potentially lead to the development of high performance devices based on discretely-supported NIL.
Non-planar morphology is a common feature of devices applied in various physical fields, such as light or fluid, which pose a great challenge for surface nano-patterning to improve their performance. The present study proposes a discretely-supported nanoimprint lithography (NIL) technique to fabricate nanostructures on the extremely non-planar surface, namely high-spatial-frequency stepped surface. The designed discretely imprinting template implanted a discretely-supported intermediate buffer layer made of sparse pillars arrays. This allowed the simultaneous generation of air-cushion-like buffer and reliable support to the thin structured layer in the template. The resulting low bending stiffness and distributed concentrated load of the template jointly overcome the contact difficulty with a stepped surface, and enable the template to encase the stepped protrusion as tight as possible. Based on the proposed discretely-supported NIL, nanostructures were fabricated on the luminous interface of light emitting diodes chips that covered with micrometer step electrodes pad. About 96% of the utilized indium tin oxide transparent current spreading layer surface on top of the light emitting diode (LED) chips was coated with nanoholes array, with an increase by more than 40% in the optical output power. The excellent ability of nanopatterning a non-planar substrate could potentially lead innovate design and development of high performance device based on discretely-supported NIL.

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