4.8 Article

Gate-Switchable Arrays of Quantum Light Emitters in Contacted Monolayer MoS2 van der Waals Heterodevices

Journal

NANO LETTERS
Volume 21, Issue 2, Pages 1040-1046

Publisher

AMER CHEMICAL SOC
DOI: 10.1021/acs.nanolett.0c04222

Keywords

single-photon emitters; field-effect device; nanoscale optoelectronic devices; 2D materials; van der Waals heterostack

Funding

  1. Deutsche Forschungsgemeinschaft (DFG) via the Munich Center for Quantum Science and Technology (MCQST) [EXC-2111390814868, EXC 2089/1-390776260]
  2. European Union [820423 (S2QUIP)]
  3. German Federal Ministry of Education and Research via the funding program Photonics Research Germany [13N14846]
  4. Bavarian Academy of Sciences and Humanities
  5. Alexander von Humboldt Foundation
  6. Goran Gustafsson Foundation (SweTeQ)
  7. Deutsche Forschungsgemeinschaft (DFG) [RTG 2247]
  8. TUM International Graduate School of Science and Engineering (IGSSE)
  9. Swedish Research Council [201606122]
  10. Elemental Strategy Initiative
  11. MEXT, Japan [JPMXP0112101001]
  12. JSPS KAKENHI [JP20H00354]
  13. CREST, JST [JPMJCR15F3]

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The researchers demonstrated electrostatic switching of individual, site-selectively generated matrices of single photon emitters in MoS2 van der Waals heterodevices, showing a first step towards producing scalable, gate-addressable, and gate-switchable arrays of quantum light emitters in MoS2 heterostacks.
We demonstrate electrostatic switching of individual, site-selectively generated matrices of single photon emitters (SPEs) in MoS2 van der Waals heterodevices. We contact monolayers of MoS2 in field-effect devices with graphene gates and hexagonal boron nitride as the dielectric and graphite as bottom gates. After the assembly of such gate-tunable heterodevices, we demonstrate how arrays of defects, that serve as quantum emitters, can be site-selectively generated in the monolayer MoS2 by focused helium ion irradiation. The SPEs are sensitive to the charge carrier concentration in the MoS2 and switch on and off similar to the neutral exciton in MoS2 for moderate electron doping. The demonstrated scheme is a first step for producing scalable, gate-addressable, and gate-switchable arrays of quantum light emitters in MoS2 heterostacks.

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