4.8 Article

Van der Waals Multiferroic Tunnel Junctions

Journal

NANO LETTERS
Volume 21, Issue 1, Pages 175-181

Publisher

AMER CHEMICAL SOC
DOI: 10.1021/acs.nanolett.0c03452

Keywords

Multiferroic tunnel junctions; van der Waals materials; tunneling electroresistance; tunneling magnetoresistance; multiple nonvolatile resistance states; resistance-area product

Funding

  1. National Natural Science Foundation of China [11704135, 61674062, 61821003]

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This study investigates the spin-dependent transport properties of van der Waals multiferroic tunnel junctions (MFTJs) composed of 2D ferromagnetic FemGeTe2 electrodes and 2D ferroelectric In2Se3 barrier layers. The proposed vdW MFTJs demonstrate multiple nonvolatile resistance states associated with the polarization orientation of the ferroelectric layer and magnetization alignment of the ferromagnetic layers, with a remarkably low resistance-area product making them promising for nonvolatile memory applications.
Multiferroic tunnel junctions (MFTJs) have aroused significant interest due to their functional properties useful for nonvolatile memory devices. So far, however, all of the existing MFTJs have been based on perovskite-oxide heterostructures limited by a relatively high resistance-area (RA) product unfavorable for practical applications. Here, using first-principles calculations, we explore spin-dependent transport properties of van der Waals (vdW) MFTJs which consist of two-dimensional (2D) ferromagnetic FemGeTe2 (n = 3, 4, 5) electrodes and 2D ferroelectric In2Se3 barrier layers. We demonstrate that such FemGeTe2/In2Se3/FenGeTe2 (n = 3, 4, 5; m # n) MFTJs exhibit multiple nonvolatile resistance states associated with different polarization orientation of the ferroelectric In2Se3 layer and magnetization alignment of the two ferromagnetic FenGeTe2 layers. We find a remarkably low RA product (less than 1 Omega.mu m(2)) which makes the proposed vdW MFTJs superior to the conventional MFTJs in terms of their promise for nonvolatile memory applications.

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