Approximated expression of the hygroscopic growth factor for polydispersed aerosols

Hygroscopic growth of aerosols plays an important role in the characterization of atmospheric aerosols. Physico-chemical and optical properties of aerosols are dependent on relative humidity (RH) as well as on their size and composition. In this study, scattering enhancement factors, f (RH), for polydispersed aerosols were approximated. f(RH) of ammonium sulfate and ammonium nitrate (AS) and NaCl aerosols (ss) were considered under the assumption of externally mixed aerosols. f(RH) was calculated using the Mie theory for polydispersed aerosols at a given RH and corresponding water uptake (denoted as fMie(RH)). f(RH) was approximated as a quadratic function of RH (denoted as fapp(RH)). The obtained approximated f(RH) or fapp(RH)) values were compared with the values based on the Mie theory and showed a reasonable agreement between them. To the best of our knowledge, this is the first study that parametrizes the size dependency of f(RH) for log normally distributed aerosols.

Automated summary

In this study, the scattering enhancement factors f(RH) for polydispersed aerosols were approximated using the Mie theory, showing reasonable agreement with the values based on the theory. This study is the first to parameterize the size dependency of f(RH) for log normally distributed aerosols.