4.8 Article

Methane Exhaust Measurements at Gathering Compressor Stations in the United States

Journal

ENVIRONMENTAL SCIENCE & TECHNOLOGY
Volume 55, Issue 2, Pages 1190-1196

Publisher

AMER CHEMICAL SOC
DOI: 10.1021/acs.est.0c05492

Keywords

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Funding

  1. National Energy Technology Laboratory, Office of Fossil Energy [DE-FE0029068]
  2. Anadarko Petroleum Corporation
  3. Colorado Energy Research Collaboratory
  4. Colorado Energy Office
  5. DCP Midstream
  6. Kinder Morgan Natural Gas Pipelines
  7. Mark West Energy Partners
  8. ONE Future
  9. Pioneer Natural Resources
  10. Southwestern Energy
  11. Equinor
  12. Williams
  13. XTO Energy, Inc
  14. DOE [DE-FE0029084]

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A novel method was used to quantify combustion slip from natural gas compressor engines at gathering and boosting stations in the U.S. The study found that methane emission rates were lower for lean-burn engines and higher for rich-burn engines, compared to existing emission factors. Modelled results suggest that unburned methane accounts for a significant portion of methane emissions from the natural gas sector in the U.S.
Unburned methane entrained in exhaust from natural gas-fired compressor engines (combustion slip) can account for a substantial portion of station-level methane emissions. A novel in-stack, tracer gas method was coupled with Fourier transform infrared (FTIR) species measurements to quantify combustion slip from natural gas compressor engines at 67 gathering and boosting stations owned or managed by nine study partner operators in 11 U.S. states. The mean methane emission rate from 63 four-stroke, lean-burn (4SLB) compressor engines was 5.62 kg/h (95% CI = 5.15-6.17 kg/h) and ranged from 0.3 to 12.6 kg/h. The mean methane emission rate from 39 four-stroke, rich-burn (4SRB) compressor engines was 0.40 kg/h (95% CI = 0.37-0.42 kg/h) and ranged from 0.01 to 4.5 kg/h. Study results for 4SLB engines were lower than both the U.S. EPA compilation of air pollutant emission factors (AP-42) and Inventory of U.S. Greenhouse Gas Emissions and Sinks (GHGI) by 8 and 9%, respectively. Study results for 4SRB engines were 43% of the AP-42 emission factor factor, the latter of which does not distinguish between engine types. Total annual combustion and 8% of the GHGI emission slip from the U.S. natural gas gathering and boosting sector was modeled using measured emission rates and compressor unit counts from the U.S. EPA Greenhouse Gas Reporting Program. Modeled results [328 Gg/y (95% CI = 235-436 Gg/y) of unburned methane] would account for 24% (95% CI = 17-31%) of the 1391 Gg of methane emissions for Gathering and Boosting Stations, or 6% of the net emissions for Natural Gas Systems (5598 Gg) as reported in the 2020 U.S. EPA GHGI. Gathering and boosting combustion slip emissions reported in the 2020 GHGI (374 Gg) fall within the uncertainty of this model.

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