Journal
CHEMICAL ENGINEERING JOURNAL
Volume 402, Issue -, Pages -Publisher
ELSEVIER SCIENCE SA
DOI: 10.1016/j.cej.2020.126184
Keywords
Artificial synthesis; Photocatalysts; Nanomaterials; Hydrogenation; CO2 photoreduction; Photoreactors
Categories
Funding
- Creative Materials Discovery Program through the National Research Foundation of Korea (NRF) - Ministry of Science and ICT [2017M3D1A1039379]
- Basic Research Laboratory of the NRF - Korean government [2018R1A4A1022647]
- Korea Research Fellowship Program through the NRF - Ministry of Science and ICT [2020H1D3A1A04081409]
- National Research Foundation of Korea [4120200513611, 4199990514635, 2017M3D1A1039379] Funding Source: Korea Institute of Science & Technology Information (KISTI), National Science & Technology Information Service (NTIS)
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Converting solar energy into fuel via photo-assisted water splitting to generate H-2 or drive CO2 photoreduction is an attractive scientific and technological goal to address the increasing global demand for energy and to reduce the impact of energy production on climate change. Solar-driven hydrogenation of CO2 into value-added chemical products is one of the most promising strategies for reducing CO2 and is anticipated to be a sustainable energy source shortly. In this study, we focus on the utilization of different sustainable H-2 sources for the photoreduction of CO2 to value-added organic products. Various photocatalysts, photoreactor configurations, and reaction parameters for the photoreduction of CO(2 )are discussed. For future research endeavors, a general approach for the photoreduction of CO2 to mimic natural photosynthesis, in which the H-2 source is provided directly during the photocatalytic water splitting, is proposed and verified to generate value-added organic products successfully.
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