4.7 Article

Marine biomass-derived composite aerogels for efficient and durable solar-driven interfacial evaporation and desalination

Journal

CHEMICAL ENGINEERING JOURNAL
Volume 417, Issue -, Pages -

Publisher

ELSEVIER SCIENCE SA
DOI: 10.1016/j.cej.2020.128051

Keywords

Marine biomass; Ulva prolifera; Solar interfacial evaporation; Solar desalination; Water purification

Funding

  1. Qingdao Science and Technology Program: Youth Project of Applied Basic Research, China [19-6-2-15-cg]
  2. Fundamental Research Funds for the Central Universities, China [201941011]
  3. Taishan Scholar Program of Shandong Province, China [tsqn201812026]
  4. Shandong Provincial Natural Science Foundation of China [ZR2019QB014]
  5. Natural Science Foundation of China [41906126, 41976117]

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This study successfully extracted nanocellulose (NC) from seaweed and developed durable composite aerogels with efficient water evaporation rate for use in interfacial steam generators. The research demonstrates a new approach of utilizing marine biomass to manufacture high-performance interfacial steam generators, promoting the combination of clean water production and sustainable development of marine ecosystems.
Solar-driven interfacial evaporation is an emerging and sustainable technology with growing potential for applications in water distillation and desalination. Despite the ongoing progress in clean water production, the high cost, delicate structures, leaching and disposal of synthetic materials remain the major roadblocks toward large-scale and real-world applications. Herein, nanocellulose (NC) is successfully extracted from abundant, inexhaustible and biodegradable biomass Ulva (Enteromorpha) prolifera that collected from the coast of Qingdao, China. Incorporation of polyvinyl alcohol (PVA) into the NC scaffolds and subsequent cross-linking endow the composite aerogels with efficient water diffusion, enhanced mechanical strength and good deformation resistance. The cross-linked composite aerogels can serve as main structural elements and integrate a monolithic, self-floating and durable steam generator. Under one sun, the good water evaporation rate of 1.4 kg m(-2) h(-1) is among the best-performing interfacial steam generators constructed by using cellulose-based materials as structural components. This study demonstrates a new concept of using marine (blue) biomass-derived NC as crude material and building block to construct high-performance and durable interfacial steam generators, synergistically considering clean water production and sustainability of marine ecosystems.

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