Journal
BULLETIN OF THE CHEMICAL SOCIETY OF JAPAN
Volume 94, Issue 4, Pages 1215-1231Publisher
CHEMICAL SOC JAPAN
DOI: 10.1246/bcsj.20200389
Keywords
Covalent organic frameworks; Two-dimensional polymers; Design and synthesis
Categories
Funding
- MOE tier 1 grant [R-143-000A71-114]
- NUS start-up grant [R-143-000-A28-133]
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This paper discusses the characteristics of covalent organic frameworks as a class of polymer materials and their applications in the design of organic/polymeric materials. By studying the interactions between ordered structures and different particles, unique structural features and functions specific to covalent organic frameworks have been discovered.
Covalent organic frameworks comprise a class of polymer which covalently links organic units into well-defined architectures to create ordered structures and offers an irreplaceable platform for designing organic/polymeric materials. In this award account, we trace our paths and show our initiatives to explore this class of molecular frameworks, by establishing design principle and synthetic strategies and developing functions and properties. By elucidating interplays of ordered structures with photons, excitons, electrons, holes, ions and molecules, we scrutinize unique structural features and functions which are specific to the ordered structures. We predict the key fundamental issues to be addressed in future and show the directions from perspectives of chemistry, physics, and materials science.
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